Variation of diamondoid compounds in the fuel oil during long-term natural weathering
YANG Bai-juan1,2, YAO Peng1, YU Zhi-gang1
1. Key Laboratory of Marine Chemistry Theory and Technology, Ministry of Education, Department of Chemistry and Chemical Engineering, Ocean University of China, Qingdao 266100, China;
2. Research Center for Marine Ecology, The First Institute of Oceanography, SOA, Qingdao 266061, China
Abstract：The changes of diamondoid compounds in the fuel oil sample during natural long-term weathering (0~100 days) were presented.Adamantanes in fuel oil were not found after 60 day natural weathering,adamantanes in crude oil from Bohai sea No.1 were not found after 45 day natural weathering.The concentrations of diamantanes slightly decrease with an increase of weathering time and diamantanes have stronger weathering-resistant capabilities.According to the "Student's t" test,seven ratios of diamantanes had no apparent changes which could indicate the source of the samples during 20 days weathering.Diamantanes ratios of DMDI-3,DMDI-4 and DMDI-5 are essentially unaltered after 100 days natural weathering which could indicate the source of the samples during natural long-term weathering.The diagnostic ratios of diamantanes in fuel oil are relatively more stable compare with those in crude oil.
YANG Bai-juan,YAO Peng,YU Zhi-gang. Variation of diamondoid compounds in the fuel oil during long-term natural weathering[J]. Marine Environmental Science, 2016, 35(5): 697-702.
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